Does the documents folder need to be in the onedrive personal folder

[Windows 11]

Recently got the family computer back from the geek squad after getting some upgrades on it. Our computer now has 2tb of memory with about 1.44 free, but the onedrive isn't allowing me to sync any of my files (it's sims custom content mostly) or add any new packages to my mods folder. The documents folder is located in the "personal" folder(?) that I'm assuming is the onedrive since it has the little cloud icon next to it. I thought buying a membership would increase the available storage on the drive itself but realized too late that it was actually for their cloud storage. I'm way over the 5

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